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11.
Min Mao Jing Xu Lingjiao Li Sheng Zhao Xuanhao Li 《International Journal of Hydrogen Energy》2021,46(45):23190-23204
Using sunlight to catalyze water to produce H2 is a key technology to solve the problem of energy shortage. In this research, perovskite-type NiMnO3 and Ni3S4 was recombined through secondary hydrothermal treatment. The optimal hydrogen evolution for composite materials NiMnO3/Ni3S4is 3.76 μmol mg?1 h?1, that 3.7 and 4 times more than that of two monomer materials, respectively. After four cycles of catalytic experiments, proving the high efficiency and stability of the composite catalyst. The characteristics of fluorescence spectroscopy and electrochemistry have confirmed the existence of p-n heterostructures, the excellent catalytic performance is related to the built-in electric field (accelerating the separation and utilization of photocharges) generated by the combination of NiMnO3 and Ni3S4. Strengthening the performance of the catalyst by constructing a heterostructure is an effective modification strategy and has positive application value in the fields of sensors and optoelectronics. 相似文献
12.
Ning Wang Yinya Li Guoqing Qi Andong Sheng 《International Journal of Adaptive Control and Signal Processing》2019,33(7):1174-1188
This paper investigates the state estimation issue for a class of wireless sensor networks (WSNs) with the consideration of limited energy resources. First, a multirate estimation model is established, and then, a new event‐triggered two‐stage information fusion algorithm is developed based on the optimal fusion criterion weighted by matrices. Compared with the existing methods, the presented fusion algorithm can significantly reduce the communication cost in WSNs and save energy resources of sensors efficiently. Furthermore, by presetting a desired containment probability over the interval [0,1] with the developed event‐triggered mechanism, one can obtain a suitable compromise between the communication cost and the estimation accuracy. Finally, a numerical simulation for the WSN tracking system is given to demonstrate the effectiveness of the proposed method. 相似文献
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Raul D. Rodriguez Sergey Shchadenko Gennadiy Murastov Anna Lipovka Maxim Fatkullin Ilia Petrov Tuan-Hoang Tran Alimzhan Khalelov Muhammad Saqib Nelson E. Villa Vladimir Bogoslovskiy Yan Wang Chang-Gang Hu Alexey Zinovyev Wenbo Sheng Jin-Ju Chen Ihsan Amin Evgeniya Sheremet 《Advanced functional materials》2021,31(17):2008818
Polyethylene terephthalate (PET) is the most widely used polymer in the world. For the first time, the laser-driven integration of aluminum nanoparticles (Al NPs) into PET to realize a laser-induced graphene/Al NPs/polymer composite, which demonstrates excellent toughness and high electrical conductivity with the formation of aluminum carbide into the polymer is shown. The conductive structures show an impressive mechanical resistance against >10000 bending cycles, projectile impact, hammering, abrasion, and structural and chemical stability when in contact with different solvents (ethanol, water, and aqueous electrolytes). Devices including thermal heaters, carbon electrodes for energy storage, electrochemical and bending sensors show this technology's practical application for ultra-robust polymer electronics. This laser-based technology can be extended to integrating other nanomaterials and create hybrid graphene-based structures with excellent properties in a wide range of flexible electronics’ applications. 相似文献
15.
Liu Yang Pengfei Yu Wenyuan Li Fengliang Cao Xin Jin Sheng Xue Xianglong Zhang Tingwei Zhang Mingbo Wu Wenting Wu 《American Institute of Chemical Engineers》2022,68(9):e17760
Hydrogen peroxide (H2O2) has been listed as one of the 100 most important chemicals in the world. However, huge amount of residual H2O2 is hard to timely decomposed into O2 and H2O under acidic condition, easily resulting in explosion hazard. Here, we reported a core–shell structure catalyst, that is graphene with Co N structure encapsulated Co nanoparticles. Co N graphene shell serves as the active site for the H2O2 decomposition, and Co core further enhance this decomposition. Benefiting from it, the H2O2 decomposition were close to 100% after 6 cycles without pH adjustment, which increased 6 orders of magnitude compared with no catalyst. At the same time, the O2 generation reached 99.67% in 2 h with little metal leaching, and ·OH has been greatly inhibited to only 0.08%. This work can cleanly remove H2O2 with little deep oxidation and protect the process of H2O2 utilization to achieve a safer world. 相似文献
16.
Jun-Hao Liu Zhuang Ge Qian Wang Geng Wang Li-Na Sheng Wen-Wen Ge Xing Xu Peng Shuai Qi Zeng Bo Wu 《核技术(英文版)》2019,30(10)
A foil–microchannel plate(MCP) detector,which uses electrostatic lenses and possesses both good position and timing resolutions, has been designed and simulated for beam diagnostics and mass measurements at the next-generation heavy-ion-beam facility HIAF in China. Characterized by low energy loss and good performances of timing and position measurements, it would be located at focal planes in fragment separator HFRS for position monitoring, beam turning, Bρ measurement, and trajectory reconstruction. Moreover, it will benefit the building-up of a magnetic-rigidity–energy-loss–time-offlight(Bρ-△E-TOF) method at HFRS for high-precision in-flight particle identification of radioactive isotope beams on an event-by-event basis. Most importantly, the detector can be utilized for in-ring TOF and position measurements,beam-line TOF measurements at two achromatic foci, and position measurements at a dispersive focus of HFRS, thus making it possible to use two complementary mass measurement methods [isochronous mass spectrometry at the storage ring SRing and magnetic-rigidity–time-of-flight(Bρ-TOF) at the beam-line HFRS] in one single experimental run. 相似文献
17.
Wen Sheng Du 《国际智能系统杂志》2019,34(11):2835-2862
Weighted power means with weights and exponents serving as their parameters are generalizations of arithmetic means. Taking into account decision makers' flexibility in decision making, each attribute value is usually expressed by a -rung orthopair fuzzy value ( -ROFV, ), where the former indicates the support for membership, the latter support against membership, and the sum of their th powers is bounded by one. In this paper, we propose the weighted power means of -rung orthopair fuzzy values to enrich and flourish aggregations on -ROFVs. First, the -rung orthopair fuzzy weighted power mean operator is presented, and its boundedness is precisely characterized in terms of the power exponent. Then, the -rung orthopair fuzzy ordered weighted power mean operator is introduced, and some of its fundamental properties are investigated in detail. Finally, a novel multiattribute decision making method is explored based on developed operators under the -rung orthopair fuzzy environment. A numerical example is given to illustrate the feasibility and validity of the proposed approach, and it is shown that the power exponent is an index suggesting the degree of the optimism of decision makers. 相似文献
18.
Zehui Zhang Ting Li Yingying Sheng Lei Liu Hai‐Chen Wu 《Small (Weinheim an der Bergstrasse, Germany)》2019,15(2)
Cancer biomarkers are expected to be indicative of the occurrence of certain cancer diseases before the tumors form and metastasize. However, many biomarkers can only be acquired in extremely low concentrations, which are often beyond the limit of detection (LOD) of current instruments and technologies. A practical strategy for nanopore sensing of cancer biomarkers in raw human blood down to the femtomolar level is developed here. This strategy first converts the detection of cancer biomarkers to the quantification of copper ions by conducting a sandwich assay involving copper oxide nanoparticles. The released Cu2+ is then taken to catalyze the “click” reaction which ligates a host–guest modified DNA probe. Finally, this DNA probe is subjected to single‐channel recordings to afford the translocation events that can be used to derive the concentrations of the original biomarkers. Due to the amplification effects of nanoparticle loadings and the “click” reaction, the LOD of this strategy can be as low as the subfemtomolar level. Further, the acid treatment step could effectively eliminate the interferences from plasma proteins in raw human blood and make the strategy highly suitable for the detection of cancer biomarkers in clinical samples. 相似文献
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